PiHole Can't Resolve 'ns1.pi-hole.net' and Other Issues

NOT sure, however, check this, common problem with bullseye & unbound...

WARNING: Raspbian October 2021 release bullseye + unbound - General / Customizing Pi-hole - Pi-hole Userspace

TLDR;
comment out the unbound entry in /etc/resolvconf.conf, however, if resolvconf managed to run with the entry active , it creates a file /etc/unbound/unbound.conf.d/resolvconf_resolvers.conf. You need to delete that file and restart unbound to resume normal behaviour.