Pi-Hole Webpages no longer load

Your debug log shows your lighttpd web server is not running:

*** [ DIAGNOSING ]: Pi-hole processes
[✗] lighttpd daemon is failed

You may test your lighttpd installation for syntactical correctness by running:

lighttpd -t -f /etc/lighttpd/lighttpd.conf

If that comes back with Syntax OK, try restarting it:

sudo service lighttpd restart

In case that fails, please provide the output for:

sudo systemctl status --full --no-pager lighttpd.service

All above commands need to be run on your Pi-hole machine.

EDIT:
Since you are running on Orange Pi, probably also check your ramlog ownerships as mentioned in Cannot access web interface - #8 by DanSchaper.