That ...
On computer with ChromeOS installed ...
Will Pi-Hole work properly ...
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If you're asking whether ChromeOS can use Pi-hole on the LAN or whether it ignores it, past behaviour shows that ChromeOS will respect the network like any other client, so if it picks up an IP via DHCP it will use the DNS servers indicated.
If you're asking whether it's possible to install Pi-hole on ChromeOS, well that is not a supported OS (as has already been explained on GitHub).
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